Bootstrap 3
HTML
<script src="//netdna.bootstrapcdn.com/bootstrap/3.1.1/js/bootstrap.min.js"></script>
<link rel="stylesheet" href="//netdna.bootstrapcdn.com/bootstrap/3.1.1/css/bootstrap.min.css">
<div class="form-body">
<div class="row">
<div class="col-md-2">
<div class="form-group">
<label class="radio-inline">
<input type="radio" ID="optRequestImmediate" runat="server">Immediately</input>
</label>
<label class="radio-inline">
<input type="radio" ID="optRequestAt" runat="server">At:</input>
</label>
</div>
</div>
<div class="col-md-2">
<div class="form-group">
<label>Request Date</label>
<input ID="txtRequestDate" Class="form-control date" runat="server"></input>
</div>
</div>
<div class="col-md-2">
<div class="form-group">
<label>Request Time</label>
<input ID="txtRequestTime" Class="form-control time" runat="server"></input>
</div>
</div>
<div class="col-md-4">
<div class="form-group">
<button ID="btnRequest" Class="btn green" Text="Request Synchronization">Request Synchronization</button>
</div>
</div>
</div>
</div>
CSS
.big-box, .small-box {
border: 1px solid red;
}